If the purpose of the borrowing was to acquire (or refinance) a let property then the interest is deductible even if the borrowing is secured on your home.
The new mortgage on your home is being used to refinance the existing mortgage on your home (1) and the existing homeowner loan secured on your home that you have used to refinance the original mortgage on your let property (2). Some, including me, would say that you are entitled to claim a deduction for part of this interest to the extent that it attributable to refinancing 2. However, another view is that none of the interest is dedcutible because it fails the "wholly and exclusively" test by reason of refinancing 1.
savva0122 wrote:Am I allowed to increase the amount I currently claim interest relief to £140k from the £57k?
Only if the "extra" £83k has been used to refinance (i.e. pay off existing debt) to acquire your let property. You could borrow against the let property, taking advantage of its increased value, and then use funds from teh new mortgage on your home to repay that buy-to-let borrowing. That would enable you to calim a tax deduction by reference to teh increased value but clearly there would be costs to doing so because of teh additional interim borroowing. What you propose may give the same end result but you would be short-cutting vital steps to get there and the tax anaylsis would be different as a consequence.